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1.
A photochemical scheme which includes a detailed treatment of multiple scattering up to solar zenith angles of 96° (developed for use in a GCM) has been used to study partitioning within chemical families. Attention is drawn to the different zenith angle dependence of diffuse radiation for the two spectral regions <310 nm and >310 nm. The effect that this has on the so-called 40 km ozone problem is discussed. The importance of correctly including multiple scattering for polar ozone studies is emphasised. 相似文献
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The radiometers on board the satellites ERS-1, TOPEX/Poseidon, ERS-2, GFO, Jason-1, and Envisat measure brightness temperatures at two or three different frequencies to determine the total columnal water vapor content and wet tropospheric path delay, a major correction to the altimeter range measurements. In order to asses the long-term stability of the path delay, the radiometers are calibrated against vicarious cold and hot references, against each other, and against several atmospheric models. Four of these radiometers exhibit significant drifts in at least one of the channels, resulting in yet unmodeled errors in path delay of up to 1 mm/year, thus limiting the accuracy at which global sea level rise can be inferred from the altimeter range measurements. 相似文献
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Carbonyl products have been identified and their formation yields measured in experiments involving the gas phase reaction of ozone with 1,1-disubstituted alkenes at ambient T and p=1 atm. of air. Sufficient cyclohexane was added to scavenge the hydroxyl radical in order to minimize OH-alkene and OH-carbonyl reactions. Formation yields (carbonyl formed/ozone reacted) of primary carbonyls were close to the value of 1.0 that is consistent with the mechanism: O3+R1R2C=CH2 (HCHO+R1R2COO)+(1–)(R1COR2+H2COO) where formaldehyde and the ketone R1 COR2 are the primary carbonyls and R1R2COO and H2COO are the corresponding biradicals. Measured values of were 0.58–0.82 and indicate modest preferential formation of formaldehyde and the disubstituted biradical as compared to the ketone and the biradical H2COO. Carbonyls other than the primary carbonyls were identified. Their formation is discussed in terms of subsequent reactions of the disubstituted biradicals R1R2COO. Similarities and differences between disubstituted and monosubstituted biradicals are outlined. 相似文献
6.
利用华中区域代表性站点金沙国家大气本底站2007—2018年的PM2.5、PM10颗粒物质量浓度数据,2019年3月—2019年6月反应性气体数据,对华中区域空气质量进行整体评价,并分析了颗粒物浓度的变化特征及其影响因素。结果表明,反应性气体CO、SO2、NO、NO2质量浓度其日平均最大值、平均值均达到一级标准,O3日平均值超标率为10.6%,PM2.5超标率为18%,PM10超标率为17%。从颗粒物质量浓度多年变化来看,2007—2013年金沙站大气颗粒物质量浓度属于上升趋势,2013年至今质量浓度呈现下降趋势,风向风速也在一定程度上影响颗粒物的来源。 相似文献
7.
Bruce A. Callander 《GeoJournal》1997,42(1):55-63
IPCCs statement in its 1995 report (IPCC 1996) that a human influence was discernible in global climate has been widely quoted but often misunderstood. The character of the evidence underpinning this detection statement is explained so that its strengths and weaknesses can be better understood and the subtleties of its message better appreciated. To demonstrate the close linkage between the government-approved summary and the underlying chapters of the IPCC report the detailed evolution of the detection statement from first draft through to the form finally approved by the IPCC is described. 相似文献
8.
Günter Helas Jürgen Lobert Dieter Scharffe Luise Schäfer Johann Goldammer Jean Baudet Brou Ahoua Ayité-Lô Ajavon Jean-Pierre Lacaux Robert Delmas Meinrat O. Andreae 《Journal of Atmospheric Chemistry》1995,22(1-2):163-174
Ozone has been observed in elevated concentrations by satellites over areas previously believed to be background. There is meteorological evidence, that these ozone plumes found over the Atlantic Ocean originate from vegetation fires on the African continent.In a previous study (DECAFE-88), we have investigated ozone and assumed precursor compounds over African tropical forest regions. Our measurements revealed large photosmog layers at altitudes from 1.5 to 4 km. Both chemical and meteorological evidence point to savanna fires up to several thousand km upwind as sources.Here we describe ozone mixing ratios observed over western Africa and compare ozone production ratios from different field measurement campaigns related to vegetation burning. We find that air masses containing photosmog ingredients require several days to develop their oxidation potential, similar to what is known from air polluted by emissions from fossil fuel burning. Finally, we estimate the global ozone production due to vegetation fires and conclude that this source is comparable in strength to the stratospheric input. 相似文献
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Hajduk, et al (1992) have drawn attention to a possible source of error in our earlier analysis of visual and radar observations of shower meteors from which we calculated the ozone concentration at meteor heights. We have considered their main criticism that the features of our data which we used to calculate the ozone concentration may have been due to the constraint that our meteors had to be observed by both methods. We have shown that observations collected from radar-only systems show very similar characteristics and that these can be analysed without recourse to visual data to produce very similar results to those from our original analysis.
Presented at theInternational Conference on Meteoroids 23 – 31 August 1994 in Bratislava.Submitted to Earth, Moon and Planets 相似文献
10.
根据Dobson和TOMS资料分析北京和昆明大气臭氧总量变化特征 总被引:11,自引:0,他引:11
用约20年 Dobson和TOMS资料来分析北京(39.93°N,116.40°E)和昆明 (25.02°N,102.68°)两地大气臭氧总量的变化特征,结果表明:(1)在1979-2000年间北京大气臭氧长期变化趋势是-0.642 DU/年,而昆明在1980-2000年间的趋势是-0.009 DU/年;(2)北京和昆明两地大气臭氧都有很强的季节内变化(尤其冬季更强),与季节性变化强度相当;(3)在北京和昆明,由记录较短的大气臭氧资料分析得到的长期变化趋势,与较长记录得到的结果有显著差异;(4)在北京(中纬度)和昆明(低纬度)大气臭氧都有显著的准两年振荡信号;(5)两个站点大气臭氧的年际变化主要由长期趋势项和准两年振荡信号组成;(6)Dobson仪测量得到的臭氧总量与TOMS资料非常一致。 相似文献